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21.
Shohei Minagawa Shoji Fujiwara Takeshi Hashimoto Takashi Hayashita 《International journal of molecular sciences》2021,22(9)
Cyclodextrins (CyDs) are water-soluble host molecules possessing a nanosized hydrophobic cavity. In the realm of molecular recognition, this cavity is used not only as a recognition site but also as a reaction medium, where a hydrophobic sensor recognizes a guest molecule. Based on the latter concept, we have designed a novel supramolecular sensing system composed of Zn(II)-dipicolylamine metal complex-based azobenzene (1-Zn) and 3A-amino-3A-deoxy-(2AS,3AS)-γ-cyclodextrin (3-NH2-γ-CyD) for sensing adenosine-5′-triphosphate (ATP). 1-Zn showed redshifts in the UV-Vis spectra and induced circular dichroism (ICD) only when both ATP and 3-NH2-γ-CyD were present. Calculations of equilibrium constants indicated that the amino group of 3-NH2-γ-CyD was involved in the formation of supramolecular 1-Zn/3-NH2-γ-CyD/ATP. The Job plot of the ICD spectral response revealed that the stoichiometry of 1-Zn/3-NH2-γ-CyD/ATP was 2:1:1. The pH effect was examined and 1-Zn/3-NH2-γ-CyD/ATP was most stable in the neutral condition. The NOESY spectrum suggested the localization of 1-Zn in the 3-NH2-γ-CyD cavity. Based on the obtained results, the metal coordination interaction of 1-Zn and the electrostatic interaction of 3-NH2-γ-CyD were found to take place for ATP recognition. The “reaction medium approach” enabled us to develop a supramolecular sensing system that undergoes multi-point interactions in water. This study is the first step in the design of a selective sensing system based on a good understanding of supramolecular structures. 相似文献
22.
如何融合多方因素准确地为用户提供个性化产品一直是关注的热点问题,由此,一个新的近相邻改进算法融入了大众化认同度和个性化认同度,利于更加高效地挖掘隐藏信息。实验结果表明,相对于传统近相邻算法,认同度修正算法虽然查全率小幅度上下波动,但其他多个评价指标都得到极大提升,假正率和深度有所减少,查准率、[F1]值和提升度得以增加,并且,受试者特征曲线和提升曲线也都说明此修正算法具有更为显著的推荐效果。 相似文献
23.
24.
Modal analysis is an important tool in the structural dynamics community; it is widely utilised to understand and investigate the dynamical characteristics of linear structures. Many methods have been proposed in recent years regarding the extension to nonlinear analysis, such as nonlinear normal modes or the method of normal forms, with the main objective being to formulate a mathematical model of a nonlinear dynamical structure based on observations of input/output data from the dynamical system. In fact, for the majority of structures where the effect of nonlinearity becomes significant, nonlinear modal analysis is a necessity. The objective of the current paper is to demonstrate a machine learning approach to output‐only nonlinear modal decomposition using kernel independent component analysis and locally linear‐embedding analysis. The key element is to demonstrate a pattern recognition approach which exploits the idea of independence of principal components from the linear theory by learning the nonlinear manifold between the variables. In this work, the importance of output‐only modal analysis via “blind source” separation tools is highlighted as the excitation input/force is not needed and the method can be implemented directly via experimental data signals without worrying about the presence or not of specific nonlinearities in the structure. 相似文献
25.
图像纹理增强过程中容易丢失平滑区域纹理细节,而分数阶微分增强虽然能够非线性保留平滑区域纹理细节,但对频率分辨率敏感。针对这个问题,提出一种基于小波变换的分数阶微分纹理增强算法,应用于平扫计算机断层扫描(CT)图像的肝脏肿瘤区域的纹理增强。首先,通过小波变换将图像感兴趣区分解成多个子带分量;其次,基于分数阶微分定义构造一个带补偿参数的分数阶微分掩膜;最后,使用该掩膜与每个高频子带分量进行卷积并利用小波逆变换重组图像感兴趣区。实验结果表明,该方法在使用较大分数阶次显著增强肿瘤区域的高频轮廓信息的同时,有效地保留了低频平滑的纹理细节:增强后的肝细胞癌区域与原区域相比,信息熵平均增加36.56%,平均梯度平均增加321.56%,平均绝对差值平均为9.287;增强后的肝血管瘤区域与原区域相比,信息熵平均增加48.77%,平均梯度平均增加511.26%,平均绝对差值平均为14.097。 相似文献
26.
空间非合作目标位姿测量是空间在轨维护的前提。面向空间机械手对空间载体自动抓捕的应用需求,提出了基于结构光的空间非合作目标视觉测量方法。该方法以双套双线结构光测量装置作为测量传感器,以空间载体上普遍存在的星箭对接环作为抓捕目标。根据对接环的共同特点,选择直线特征和点特征相结合作为相对位姿的求解特征;基于直线特征求解圆环平面法向量,基于点特征求解圆环圆心坐标,进而得到机械手工具坐标系与对接环坐标系间的相对位姿关系;基于多重几何约束实现了不同光照条件下图像上目标直线的鲁棒识别。建立了演示验证实验系统,在大量演示实验的基础上,进行了实验结果分析。 相似文献
27.
《Digital Communications & Networks》2019,5(1):34-39
This paper proposes a novel Multiple-Input Multiple-Output (MIMO) transmission scheme based on Pattern Recognition (PR), which is termed as the PR aided Transmission Antenna Selection MIMO (PR-TAS aided MIMO). As the conventional TAS algorithms need to search all possible legitimate antenna subsets, they may impose some redundant calculations. In order to avoid this problem, we employ some pattern recognition methods to carry out the TAS algorithm in this paper. To be specific, two PR algorithms, namely the K-Nearest Neighbor (KNN) algorithm and the Support Vector Machine (SVM) algorithm, are introduced and redesigned to obtain a TAS with lower complexity but higher efficiency. Moreover, in order to improve the performance of the SVM, we propose a new feature extraction of channel matrix for the TAS. Our simulation results show that the proposed KNN and SVM based PR-TAS algorithms are capable of striking a flexible tradeoff between the complexity and the Bit Error Rate (BER), and the new feature can effectively improve the BER performance compared with the conventional feature extraction method. 相似文献
28.
Yue Zhao Jianjian Yue Wei Song Xiaona Xu Xiali Li Licheng Wu Qiang Ji 《计算机、材料和连续体(英文)》2019,60(3):1223-1235
Tibetan language has very limited resource for conventional automatic speech recognition so far. It lacks of enough data, sub-word unit, lexicons and word inventories for some dialects. And speech content recognition and dialect classification have been treated as two independent tasks and modeled respectively in most prior works. But the two tasks are highly correlated. In this paper, we present a multi-task WaveNet model to perform simultaneous Tibetan multi-dialect speech recognition and dialect identification. It avoids processing the pronunciation dictionary and word segmentation for new dialects, while, in the meantime, allows training speech recognition and dialect identification in a single model. The experimental results show our method can simultaneously recognize speech content for different Tibetan dialects and identify the dialect with high accuracy using a unified model. The dialect information used in output for training can improve multi-dialect speech recognition accuracy, and the low-resource dialects got higher speech content recognition rate and dialect classification accuracy by multi-dialect and multi-task recognition model than task-specific models. 相似文献
29.
30.
Facial Expression Recognition (FER) is an important subject of human–computer interaction and has long been a research area of great interest. Accurate Facial Expression Sequence Interception (FESI) and discriminative expression feature extraction are two enormous challenges for the video-based FER. This paper proposes a framework of FER for the intercepted video sequences by using feature point movement trend and feature block texture variation. Firstly, the feature points are marked by Active Appearance Model (AAM) and the most representative 24 of them are selected. Secondly, facial expression sequence is intercepted from the face video by determining two key frames whose emotional intensities are minimum and maximum, respectively. Thirdly, the trend curve which represents the Euclidean distance variations between any two selected feature points is fitted, and the slopes of specific points on the trend curve are calculated. Finally, combining Slope Set which is composed by the calculated slopes with the proposed Feature Block Texture Difference (FBTD) which refers to the texture variation of facial patch, the final expressional feature are formed and inputted to One-dimensional Convolution Neural Network (1DCNN) for FER. Five experiments are conducted in this research, and three average FER rates 95.2%, 96.5%, and 97% for Beihang University (BHU) facial expression database, MMI facial expression database, and the combination of two databases, respectively, have shown the significant advantages of the proposed method over the existing ones. 相似文献